Publications

2015

Is collisionless heating in capacitively coupled plasmas really collisionless?
- Lafleur Trevor
- Chabert Pascal
Plasma Sources Science and Technology, IOP Publishing, 2015, 24 (4), pp.044002. By performing a combination of test-particle and particle-in-cell simulations, we investigate electron heating in single frequency capacitively coupled plasmas (CCPs). In agreement with previous theoretical considerations highlighted in Kaganovich et al (1996 Appl. Phys. Lett. 69 3818), we show that the level of true collisionless/stochastic heating in typical CCPs is significantly smaller than that due to collisional interactions; even at very low pressures and wide gap lengths. Fundamentally electron heating is a collisional phenomenon whereby particle collisions provide the vital phase randomization and stochastization mechanism needed to generate both a local (or ohmic) heating component, and a non-local (or hybrid) heating component. (10.1088/0963-0252/24/4/044002)
DOI : 10.1088/0963-0252/24/4/044002
Solar illumination control of ionospheric outflow above polar cap arcs
- Maes Lukas
- Maggiolo R.
- de Keyser J.
- Dandouras I.
- Fear R. C.
- Fontaine Dominique
- Haaland S.
Geophysical Research Letters, American Geophysical Union, 2015, 42 (5), pp.1304-1311. We measure the flux density, composition, and energy of outflowing ions above the polar cap, accelerated by quasi-static electric fields parallel to the magnetic field and associated with polar cap arcs, using Cluster. Mapping the spacecraft position to its ionospheric foot point, we analyze the dependence of these parameters on the solar zenith angle (SZA). We find a clear transition at SZA between 94° and 107°, with the O flux higher above the sunlit ionosphere. This dependence on the illumination of the local ionosphere indicates that significant O upflow occurs locally above the polar ionosphere. The same is found for H , but to a lesser extent. This effect can result in a seasonal variation of the total ion upflow from the polar ionosphere. Furthermore, we show that low-magnitude field-aligned potential drops are preferentially observed above the sunlit ionosphere, suggesting a feedback effect of ionospheric conductivity. (10.1002/2014GL062972)
DOI : 10.1002/2014GL062972
Numerical experiment to estimate the validity of negative ion diagnostic using photo-detachment combined with Langmuir probing
- Oudini N.
- Sirse Nishant
- Benallal R.
- Taccogna F.
- Aanesland Ane
- Bendib A.
- Ellingboe A. R.
Physics of Plasmas, American Institute of Physics, 2015, 22 (7), pp.073509. This paper presents a critical assessment of the theory of photo-detachment diagnostic method used to probe the negative ion density and electronegativity α = n-/ne. In this method, a laser pulse is used to photo-detach all negative ions located within the electropositive channel (laser spot region). The negative ion density is estimated based on the assumption that the increase of the current collected by an electrostatic probe biased positively to the plasma is a result of only the creation of photo-detached electrons. In parallel, the background electron density and temperature are considered as constants during this diagnostics. While the numerical experiments performed here show that the background electron density and temperature increase due to the formation of an electrostatic potential barrier around the electropositive channel. The time scale of potential barrier rise is about 2 ns, which is comparable to the time required to completely photo-detach the negative ions in the electropositive channel (∼3 ns). We find that neglecting the effect of the potential barrier on the background plasma leads to an erroneous determination of the negative ion density. Moreover, the background electron velocity distribution function within the electropositive channel is not Maxwellian. This is due to the acceleration of these electrons through the electrostatic potential barrier. In this work, the validity of the photo-detachment diagnostic assumptions is questioned and our results illustrate the weakness of these assumptions. (10.1063/1.4926826)
DOI : 10.1063/1.4926826
Reply to Comment on "A review on ion-ion plasmas created in weakly magnetized electronegative plasmas
- Aanesland Ane
- Bredin Jérôme
- Chabert Pascal
Plasma Sources Science and Technology, IOP Publishing, 2015, 24 (3), pp.038002. This is a reply to the comments made by Bogdanov et al on our paper entitled ?A review on ion?ion plasmas created in weakly magnetized electronegative plasmas?. We have clarified some issues regarding the electronegative plasma stratification and the definition of an ion?ion plasma, and we discuss the issue of extracting negative ions from a steady-state ion?ion plasma formed at the periphery or downstream a magnetized electronegative plasma. (10.1088/0963-0252/24/3/038002)
DOI : 10.1088/0963-0252/24/3/038002
Plasma acceleration using a radio frequency self-bias effect
- Rafalskyi D.V.
- Aanesland Ane
Physics of Plasmas, American Institute of Physics, 2015, 22 (6), pp.063502. In this work plasma acceleration using a RF self-bias effect is experimentally studied. The experiments are conducted using a novel plasma accelerator system, called Neptune, consisting of an inductively coupled plasma source and a RF-biased set of grids. The plasma accelerator can operate in a steady state mode, producing a plasma flow with separately controlled plasma flux and velocity without any magnetic configuration. The operating pressure at the source output is as low as 0.2 mTorr and can further be decreased. The ion and electron flows are investigated by measuring the ion and electron energy distribution functions both space resolved and with different orientations with respect to the flow direction. It is found that the flow of electrons from the source is highly anisotropic and directed along the ion flow and this global flow of accelerated plasma is well localized in the plasma transport chamber. The maximum flux is about 7.5·1015 ions s−1 m−2 (at standard conditions) on the axis and decreasing to almost zero at a radial distances of more than 15 cm from the flow axis. Varying the RF acceleration voltage in the range 20350 V, the plasma flow velocity can be changed between 10 and 35 km/s. The system is prospective for different technology such as space propulsion and surface modification and also interesting for fundamental studies for space-related plasma simulations and investigation of the dynamo effect using accelerated rotating plasmas. I. INTRODUCT (10.1063/1.4922065)
DOI : 10.1063/1.4922065
WEST Physics Basis
- Bourdelle C.
- Artaud J.F.
- Basiuk Vincent
- Bécoulet M.
- Brémond S.
- Bucalossi J.
- Bufferand H.
- Ciraolo G.
- Colas L.
- Corre Y.
- Courtois X.
- Decker J.
- Delpech L.
- Devynck P.
- Dif-Pradalier Guilhem
- Doerner R.P.
- Douai D.
- Dumont Rémi
- Ekedahl A.
- Fedorczak N.
- Fenzi C.
- Firdaouss M.
- Garcia J.
- Ghendrih Philippe
- Gil C.
- Giruzzi G.
- Goniche M.
- Grisolia C.
- Grosman A.
- Guilhem D.
- Guirlet R.
- Gunn J.
- Hennequin Pascale
- Hillairet J.
- Hoang T.
- Imbeaux Frédéric
- Ivanova-Stanik Irena
- Joffrin E.
- Kallenbach A.
- Linke J.
- Loarer T.
- Lotte P.
- Maget P.
- Marandet Yannick
- Mayoral M.L.
- Meyer O.
- Missirlian M.
- Mollard P.
- Monier-Garbet P.
- Moreau P.
- Nardon Eric
- Pégourié B.
- Peysson Y.
- Sabot R.
- Saint-Laurent F.
- Schneider M.
- Travère J. M.
- Tsitrone E.
- Vartanian S.
- Vermare Laure
- Yoshida M.
- Zagorski R.
- Jet Contributors
Nuclear Fusion, IOP Publishing, 2015, 55 (6), pp.063017. With WEST (Tungsten Environment in Steady State Tokamak) (Bucalossi et al 2014 Fusion Eng. Des. 89 [http://dx.doi.org/10.1016/j.fusengdes.2014.01.062] 907?12 ), the Tore Supra facility and team expertise (Dumont et al 2014 Plasma Phys. Control. Fusion 56 [http://dx.doi.org/10.1088/0741-3335/56/7/075020] 075020 ) is used to pave the way towards ITER divertor procurement and operation. It consists in implementing a divertor configuration and installing ITER-like actively cooled tungsten monoblocks in the Tore Supra tokamak, taking full benefit of its unique long-pulse capability. WEST is a user facility platform, open to all ITER partners. This paper describes the physics basis of WEST: the estimated heat flux on the divertor target, the planned heating schemes, the expected behaviour of the L?H threshold and of the pedestal and the potential W sources. A series of operating scenarios has been modelled, showing that ITER-relevant heat fluxes on the divertor can be achieved in WEST long pulse H-mode plasmas. (10.1088/0029-5515/55/6/063017)
DOI : 10.1088/0029-5515/55/6/063017
The impingement of a kHz helium atmospheric pressure plasma jet on a dielectric surface
- Guaitella Olivier
- Sobota Ana
Journal of Physics D: Applied Physics, IOP Publishing, 2015, 48 (25), pp.255202. A parametric study of the impingement of a helium kHz atmospheric pressure plasma jet on a flat glass surface was performed by means of time-resolved intensified charge-coupled device imaging. The development of the plasma on the target is linked to the plasma evolution in the source and governed by the power supply. The glass surface takes part in the elongation of the plasma jet by the virtue of two mechanisms: the local enhancement of the electric field and the supply of pre-deposited charge. The evidence for the pre-deposited charge is the formation of a sheath on the glass surface, and the faint discharge formed on the glass surface during the negative voltage slope starting at the maximum of the negative current peak. The influence of the gas flow dynamics taking into account various gas flows, incident angles and distances is more important for the behaviour of the discharge on the surface than the voltage amplitude or the geometry of the source. The capacitance of the target strongly modifies the interaction with the plasma jet and increases the deposited surface charge density, featuring a streamer-like propagation mechanism in the case of high electric field enhancement at the surface. (10.1088/0022-3727/48/25/255202)
DOI : 10.1088/0022-3727/48/25/255202
Isopropanol removal using MnXOY packed bed non-thermal plasma reactor: Comparison between continuous treatment and sequential sorption/regeneration
- Sivachandiran Loganathan
- Thévenet Frédéric
- Rousseau Antoine
Chemical Engineering Journal, Elsevier, 2015, 270, pp.327-335. MnXOY coated glass beads packed bed non-thermal plasma (NTP) reactor has been designed and operated for isopropanol (IPA) removal close to indoor air conditions. The IPA removal efficiency of continuous NTP treatment is compared with the sequential approach, i.e. adsorption of IPA on MnXOY and subsequent regeneration of the saturated MnXOY surface by non-thermal plasma. The comparison between both approaches has been achieved with the same packed bed reactor and model VOC under equivalent indoor air conditions. Firstly, based on carbon mass balance calculations, the continuous treatment has shown better performances from an IPA abatement point of view, as well as from a mineralization point of view. However, the characterization of ppb level side-products evidenced that the continuous treatment leads to a more significant release of organic side products which may impact indoor air quality. Secondly, both processes have been compared in terms of energetic costs regarding (i) IPA removal, and (ii) CO2 forma- tion. Interestingly, it is evidenced that, to treat the same amount of IPA, the sequential approach requires 14.5 times less energy than the continuous NTP treatment process. Similarly, to produce the same amount of CO2, the sequential approach consumes 10 times less energy. This comparison evidences the interest of adsorption combined with subsequent non-thermal plasma regeneration for indoor air effluent treatment. (10.1016/j.cej.2015.01.055)
DOI : 10.1016/j.cej.2015.01.055
Matched dipole probe for magnetized low electron density laboratory plasma diagnostics
- Rafalskyi D.V.
- Aanesland Ane
Physics of Plasmas, American Institute of Physics, 2015, 22 (7), pp.073504. In this paper, a diagnostic method for magnetized and unmagnetized laboratory plasma is proposed, based on impedance measurements of a short matched dipole. The range of the measured electron densities is limited to low density plasmas (10121015 m−3), where other diagnostic methods have strong limitations on the magnetic field strength and topology, plasma dimensions, and boundary conditions. The method is designed for use in both large- and small-dimension plasma (<10 cm) without or with strong non-homogeneous magnetic field, which can be undefined within the probe size. The design of a matched dipole probe allows to suppress the sheath resonance effects and to reach high sensitivity at relatively small probe dimensions. Validation experiments are conducted in both magnetized (B ∼ 170 G) and unmagnetized (B = 0) low density (7 × 1012 m−37 × 1013 m−3) low pressure (1 mTorr) 10 cm scale plasmas. The experimentally measured data show very good agreement with an analytical theory both for a non-magnetized and a magnetized case. The electron density measured by the matched dipole and Langmuir probes in the range of 7 × 1012 m−37 × 1013 m−3 show less than 30% difference. An experimentally measured tolerance/uncertainty of the dipole probe method is estimated to ±1% for plasma densities above 2 × 1013 m−3. A spatial resolution is estimated from the experiments to be about 3d, where d is the dipole diameter. The diagnostic method is also validated by comparing the measured plasma impedance curves with results of analytical modelling. (10.1063/1.4926447)
DOI : 10.1063/1.4926447
Further details on the plasma E × B staircase
- Dif-Pradalier Guilhem
- Hornung G
- Ghendrih Philippe
- Sarazin Yanick
- Clairet F
- Vermare L
- Diamond P H
- Abiteboul J
- Cartier-Michaud T
- Ehrlacher C
- Esteve D
- Garbet Xavier
- Grandgirard Virginie
- Gürcan Özgür D.
- Hennequin P
- Kosuga A
- Latu Guillaume
- Morel Pierre
- Norscini C
- Sabot R
- Storelli A.
, 2015. Turbulence in hot magnetised plasmas spontaneously has been shown to spontaneously organise on global scales into the so-called " E × B staircase ". Further characterisation of this structure is detailed below.
The Plasma E × B Staircase: Turbulence Self-Regulation through Spontaneous Flow Patterning
- Dif-Pradalier Guilhem
- Hornung G
- Ghendrih Philippe
- Clairet R
- Diamond P H
- Sarazin Yanick
- Vermare L
- Abiteboul J
- Cartier-Michaud T
- Ehrlacher C
- Estève D
- Garbet Xavier
- Grandgirard Virginie
- Gürcan Özgür D.
- Hennequin P
- Kosuga Y
- Latu Guillaume
- Morel Pierre
- Norscini C
- Sabot R
, 2015. The E × B staircase [1, 2] is a spontaneously formed, turbulence-driven self-organising pattern of quasi-regular, long-lived and localised shear flow [3] and stress layers. These layers coincide with long-lived pressure corrugations and are interspersed between regions of turbulent avalanching. The typical spacing between these layers is mesoscale, noted ∆ ∼ 25 − 30ρ i [1, 4] —in-between the turbulence auto-correlation length c ∼ 5ρ i at micro scales and the profile macroscale L 100ρ i , see e.g. Fig.2 in [1]— and sets the outer scale of the turbulent avalanching. Here ρ i is ion Larmor radius. Whilst arresting, statistically, to mesoscales the detrimental avalanching these layers, located at the " steps of the staircase " are beneficial to confinement. The E×B staircase is thus best understood as a self-organising and dynamical set of weak or permeable transport barriers. Strong mean zonal flows are generated and endure at the steps of the staircase, resulting in localised deviations of the poloidal flow from its oft-assumed neoclassical prediction [5].
3D hybrid simulations of the interaction of a magnetic cloud with a bow shock
- Turc Lucile
- Fontaine Dominique
- Savoini Philippe
- Modolo Ronan
Journal of Geophysical Research Space Physics, American Geophysical Union/Wiley, 2015, 120 (8), pp.6133-6151. In this paper, we investigate the interaction of a magnetic cloud (MC) with a planetary bow shock using hybrid simulations. It is the first time to our knowledge that this interaction is studied using kinetic simulations which include self-consistently both the ion foreshock and the shock wave dynamics. We show that when the shock is in a quasi-perpendicular configuration, the MC's magnetic structure in the magnetosheath remains similar to that in the solar wind, whereas it is strongly altered downstream of a quasi-parallel shock. The latter can result in a reversal of the magnetic field north-south component in some parts of the magnetosheath. We also investigate how the MC affects in turn the outer parts of the planetary environment, i.e., from the foreshock to the magnetopause. We find the following: (i) The decrease of the Alfvén Mach number at the MC's arrival causes an attenuation of the foreshock region because of the weakening of the bow shock. (ii) The foreshock moves along the bow shock's surface, following the rotation of the MC's magnetic field. (iii) Owing to the low plasma beta, asymmetric flows arise inside the magnetosheath, due to the magnetic tension force which accelerates the particles in some parts of the magnetosheath and slows them down in others. (iv) The quasi-parallel region forms a depression in the shock's surface. Other deformations of the magnetopause and the bow shock are also highlighted. All these effects can contribute to significantly modify the solar wind/magnetosphere coupling during MC events. (10.1002/2015JA021318)
DOI : 10.1002/2015JA021318
Equatorial noise emissions with quasiperiodic modulation of wave intensity
- Nemec F.
- Santolík O.
- Hrbackova Z.
- Pickett J. S.
- Cornilleau-Wehrlin Nicole
Journal of Geophysical Research Space Physics, American Geophysical Union/Wiley, 2015, 120, pp.2649-2661. Equatorial noise (EN) emissions are electromagnetic wave events at frequencies between the proton cyclotron frequency and the lower hybrid frequency observed in the equatorial region of the inner magnetosphere. They propagate nearly perpendicular to the ambient magnetic field, and they exhibit a harmonic line structure characteristic of the proton cyclotron frequency in the source region. However, they were generally believed to be continuous in time. We investigate more than 2000 EN events observed by the Spatio-Temporal Analysis of Field Fluctuations and Wide-Band Data Plasma Wave investigation instruments on board the Cluster spacecraft, and we show that this is not always the case. A clear quasiperiodic (QP) time modulation of the wave intensity is present in more than 5% of events. We perform a systematic analysis of these EN events with QP modulation of the wave intensity. Such events occur usually in the noon-to-dawn magnetic local time sector. Their occurrence seems to be related to the increased geomagnetic activity, and it is associated with the time intervals of enhanced solar wind flow speeds. The modulation period of these events is on the order of minutes. Compressional ULF magnetic field pulsations with periods about double the modulation periods of EN wave intensity and magnitudes on the order of a few tenths of nanotesla were identified in about 46% of events. We suggest that these compressional magnetic field pulsations might be responsible for the observed QP modulation of EN wave intensity, in analogy to formerly reported VLF whistler mode QP events. (10.1002/2014JA020816)
DOI : 10.1002/2014JA020816
Kinetic simulations of secondary reconnection in the reconnection jet
- Huang S. Y.
- Zhou M.
- Yuan Z. G.
- Fu H.S.
- He J. S.
- Sahraoui Fouad
- Aunai Nicolas
- Deng X. H.
- Fu S. Y.
- Pang Y.
- Wang D. D.
Journal of Geophysical Research Space Physics, American Geophysical Union/Wiley, 2015, 120 (8), pp.61886198. Magnetic reconnection, as one important energy dissipation process in plasmas, has been extensively studied in the past several decades. Magnetic reconnection occurring in the downstream of a primary X line is referred to as secondary reconnection. In this paper, we used kinetic simulations to investigate the secondary reconnection in detail. We found that secondary reconnection is reversed by the compression caused by the outflowing jet originating from the primary reconnection site, which results in the erosion of the magnetic island between the two X lines within ~3 ωci−1. We show the observational signatures expected in electromagnetic fields and plasma measurements in the Earth's magnetotail, associated with this mechanism. These simulation results could be applied to interpret the signatures associated with the evolution of earthward magnetic islands in the Earth's magnetotail. (10.1002/2014JA020969)
DOI : 10.1002/2014JA020969
Kinetic scale turbulence and dissipation in the solar wind: key observational results and future outlook
- Goldstein M. L.
- Wicks R. T.
- Perri S.
- Sahraoui Fouad
Philosophical Transactions of the Royal Society A: Mathematical, Physical and Engineering Sciences, Royal Society, The, 2015, 373, pp.20140147. Turbulence is ubiquitous in the solar wind. Turbulence causes kinetic and magnetic energy to cascade to small scales where they are eventually dissipated, adding heat to the plasma. The details of how this occurs are not well understood. This article reviews the evidence for turbulent dissipation and examines various diagnostics for identifying solar wind regions where dissipation is occurring. We also discuss how future missions will further enhance our understanding of the importance of turbulence to solar wind dynamics. (10.1098/rsta.2014.0147)
DOI : 10.1098/rsta.2014.0147
What is the nature of magnetosheath FTEs?
- Roux A.
- Robert Patrick
- Fontaine Dominique
- Le Contel Olivier
- Canu Patrick
- Louarn P.
Journal of Geophysical Research Space Physics, American Geophysical Union/Wiley, 2015, 120 (6), pp.4576-4595. Cluster multipoint measurements are used to study two successive magnetosheath flux transfer events (FTEs). Magnetic field lines in the leading region are found to be closed magnetospheric field lines. For event 1 these field lines are wounded up by a large current structure oriented eastward and moving poleward. Conversely, the trailing region corresponds to opened magnetic field lines. For both events the leading edge of the FTEs is a tangential discontinuity separating the magnetosheath from closed field lines. In the case of event 1 magnetosheath ions are accelerated through the FTE trailing edge via a rotational discontinuity and penetrate on closed field lines through a second discontinuity. Thus, the ion jet is accelerated equatorward of the spacecraft but the backtracking of the discontinuities and the lack of dispersion show that ion acceleration occurs at less than 2 RE from Cluster. On the other hand the extrapolation forward indicates that the FTE bulge steepens as in simulations of Dorelli and Bhattacharjee). Evidence is given for the penetration of magnetosheath ions inside the core of the FTE, on closed field lines. Magnetosheath electrons are accelerated in parallel and antiparallel directions on open and on closed field lines, thus breaking the frozen-in condition. Event 2 is also split in two distinct regions but no evidence is found for accelerated bidirectional magnetosheath electrons. For event 2 the two discontinuities at the trailing region are stacked together when they are crossed by the spacecraft, suggesting that the current splitting is a reconnection signature. (10.1002/2015JA020983)
DOI : 10.1002/2015JA020983
Nature of the MHD and Kinetic Scale Turbulence in the Magnetosheath of Saturn: Cassini Observations
- Hadid Lina
- Sahraoui Fouad
- Kiyani K. H.
- Retinò Alessandro
- Modolo Ronan
- Canu Patrick
- Masters Adam
- Dougherty Michele K.
The Astrophysical Journal Letters, Bristol : IOP Publishing, 2015, 813 (2), pp.L29. Low-frequency turbulence in Saturn's magnetosheath is investigated using in situ measurements of the Cassini spacecraft. Focus is put on the magnetic energy spectra. A set of 42 time intervals in the magnetosheath were analyzed, and three main results that contrast with known features of solar wind turbulence are reported. (10.1088/2041-8205/813/2/L29)
DOI : 10.1088/2041-8205/813/2/L29
Gyrokinetic turbulence cascade via predator-prey interactions between different scales
- Kobayashi Sumire
- Gürcan Özgür D.
Physics of Plasmas, American Institute of Physics, 2015, 22 (5), pp.050702. Gyrokinetic simulations in a closed fieldline geometry are presented to explore the physics of nonlinear transfer in plasma turbulence. As spontaneously formed zonal flows and small-scale turbulence demonstrate predator-prey dynamics, a particular cascade spectrum emerges. The electrostatic potential and the density spectra appear to be in good agreement with the simple theoretical prediction based on Charney-Hasegawa-Mima equation |||ϕ̃k|||2∼||ñk||2∝k−3/(1 k2)2, with the spectra becoming anisotropic at small scales. The results indicate that the disparate scale interactions, in particular, the refraction and shearing of larger scale eddies by the self-consistent zonal flows, dominate over local interactions, and contrary to the common wisdom, the comprehensive scaling relation is created even within the energy injection region. (10.1063/1.4920965)
DOI : 10.1063/1.4920965
Polarization analysis of CuXX-lines emitted from X-pinch
- Baronova E O
- Larour Jean
- Rosmej F B
- Khattak F y
Journal of Physics: Conference Series, IOP Science, 2015, 653, pp.012145. Soft x-ray emission from CuXX L-shell lines emitted by a dense X-pinch plasma have been investigated with high-resolution curved Bragg crystals at different angles of orientation. Single shot time integrated spectra show clear evidences of polarization for the Ne-like spectral lines 2s22p6 1S0 → 2s22p53s 1P1 (λ = 12.570 Å), 2s22p6 1S0 → 2s22p53s 3P1 (λ = 12.8277 Å). The variation of the intensity ratio of these two well-separated L-shell lines is discussed in view of its application for suprathermal electron characterization under real experimental conditions of pinch plasmas. We demonstrated that the simultaneous use of two different polarization spectrometers (means 4 Bragg crystals) permitted a high level of confidence for the analysis of the variation of the line ratios due to polarization. (10.1088/1742-6596/653/1/012145)
DOI : 10.1088/1742-6596/653/1/012145
Negative hydrogen ion production mechanisms
- Bacal M.
- Wada M.
Applied Physics Reviews, AIP Publishing, 2015, 2 (2), pp.021305. Negative hydrogen/deuterium ions can be formed by processes occurring in the plasma volume and on surfaces facing the plasma. The principal mechanisms leading to the formation of these negative ions are dissociative electron attachment to ro-vibrationally excited hydrogen/deuterium molecules when the reaction takes place in the plasma volume, and the direct electron transfer from the low work function metal surface to the hydrogen/deuterium atoms when formation occurs on the surface. The existing theoretical models and reported experimental results on these two mechanisms are summarized. Performance of the negative hydrogen/deuterium ion sources that emerged from studies of these mechanisms is reviewed. Contemporary negative ion sources do not have negative ion production electrodes of original surface type sources but are operated with caesium with their structures nearly identical to volume production type sources. Reasons for enhanced negative ion current due to caesium addition to these sources are discussed. (31 pages, 265 refs) (10.1063/1.4921298)
DOI : 10.1063/1.4921298
Gas temperature measurements in oxygen plasmas by high-resolution Two-Photon Absorption Laser-induced Fluorescence
- Booth Jean-Paul
- Marinov Daniil
- Foucher Mickaël
- Guaitella Olivier
- Bresteau D.
- Cabaret Louis
- Drag Cyril
Journal of Instrumentation, IOP Publishing, 2015, 10 (11), pp.C11003. One of the most important, and difficult to measure, parameters of laboratory discharges in molecular gases is the gas translational temperature. We propose a novel technique to measure directly, with excellent spatial and temporal resolution, the velocity distribution of ground-state atoms (oxygen atoms in this case) in plasmas from the Doppler broadening of their laser excitation spectra. The method is based on the well-known Two-Photon Laser-induced Fluorescence (TALIF) technique, but uses a specially-built pulsed tunable ultraviolet laser with very narrow bandwidth which allows the Doppler profiles to be measured with high precision. This laser consists of a pulsed Nd:YAG-pumped Ti:Sapphire ring cavity which is injection-seeded by a single-mode cw Ti:sapphire laser. The single-mode infrared output pulses are frequency quadrupled by two non-linear crystals to reach the necessary UV wavelength (226 nm, 0.2 mJ) for TALIF excitation. This technique should be applicable to a wide range of discharges, ranging from low-pressure RF plasmas for surface processing to atmospheric pressure plasmas. Results of preliminary tests on low-pressure O 2 DC discharges are presented. (10.1088/1748-0221/10/11/C11003)
DOI : 10.1088/1748-0221/10/11/C11003
TALIF measurements of oxygen atom density in the afterglow of a capillary nanosecond discharge
- Klochko A.V.
- Lemainque J.
- Booth Jean-Paul
- Starikovskaia Svetlana
Plasma Sources Science and Technology, IOP Publishing, 2015, 24 (2), pp.025010. The atomic oxygen density has been measured in the afterglow of a capillary nanosecond discharge in 2430 mbar synthetic air (N 2  : O 2 = 4 : 1) by the two-photon absorption laser-induced fluorescence (TALIF) technique, combined with absolute calibration by comparison with xenon TALIF. The discharge was initiated by a train of 30 ns FWHM pulses of alternating positivenegativepositive polarity, separated by 250 ns, with a train repetition frequency of 10 Hz. The amplitude of the first pulse was 10 kV in the cable. A flow of synthetic air through the tube provided complete gas renewal between pulse trains. The O-atom density measurements were made over the time interval200 ns2 µ s after the initial pulse. The gas temperature was determined by analysis of the molecular nitrogen second positive system optical emission spectrum. The influence of the gas temperature on the atom density measurements, and the reactions producing O atoms, are discussed. (10.1088/0963-0252/24/2/025010)
DOI : 10.1088/0963-0252/24/2/025010
Ignition of methane and n-butane containing mixtures at high pressures by pulsed nanosecond discharge
- Boumehdi M.A.
- Stepanyan S.A.
- Vanhove Guillaume
- Desgroux Pascale
- Starikovskaia Svetlana
Combustion and Flame, Elsevier, 2015, 162, pp.1336-1349. A novel experimental scheme to study the ignition of combustible mixtures at high pressures under the action of a high-voltage nanosecond discharge has been developed. The experiments were performed in the combustion chamber of a Rapid Compression Machine (RCM) with a specially designed system of electrodes. A nanosecond surface dielectric barrier discharge (SDBD) provided two-dimensional low-temperature non-equilibrium plasma in the vicinity of the end plate of the combustion chamber. Radially symmetric plasma channels triggered multi-point ignition of gas mixtures at controlled pressure and temperature. Ignition delay times and energies deposited in the gaseous mixtures by the discharge were measured for different parameters of high voltage pulse, for positive or negative high-voltage pulses. The propagation of the subsequent flame in the combustion chamber was recorded with the help of high repetition rate imaging. Preliminary numerical analysis of the ignition under the action of a pulsed nanosecond discharge has been made; it was shown that production of atomic oxygen by the discharge, will modify the ignition chemistry by perturbation of the radical pool. Experiments and calculations were performed in methaneoxygen and n-butaneoxygen mixtures with equivalence ratios between 0.3 and 1 diluted by 7076% of Ar or nitrogen for temperatures between 600 and 1000 K and pressures between 6 and 16 bar. (10.1016/j.combustflame.2014.11.006)
DOI : 10.1016/j.combustflame.2014.11.006
Highly vibrationally excited O2 molecules in low-pressure inductively-coupled plasmas detected by high sensitivity ultra-broad-band optical absorption spectroscopy
- Foucher Mickaël
- Marinov Daniil
- Carbone Emile
- Chabert Pascal
- Booth Jean-Paul
Plasma Sources Science and Technology, IOP Publishing, 2015, 24 (4), pp.042001. Inductively-coupled plasmas in pure O 2 (at pressures of 5?80?mTorr and radiofrequency power up to 500?W) were studied by optical absorption spectroscopy over the spectral range 200?450?nm, showing the presence of highly vibrationally excited O 2 molecules (up to v? = 18) by Schumann?Runge band absorption. Analysis of the relative band intensities indicates a vibrational temperature up to 10,000?K, but these hot molecules only represent a fraction of the total O 2 density. By analysing the (11-0) band at higher spectral resolution the O 2 rotational temperature was also determined, and was found to increase with both pressure and power, reaching 900?K at 80?mTorr 500?W. These measurements were achieved using a new high-sensitivity ultra-broad-band absorption spectroscopy setup, based on a laser-plasma light source, achromatic optics and an aberration-corrected spectrograph. This setup allows the measurement of weak broadband absorbances due to a baseline variability lower than 2???×???10 ?5 across a spectral range of 250?nm. (10.1088/0963-0252/24/4/042001)
DOI : 10.1088/0963-0252/24/4/042001
Control and optimization of the slope asymmetry effect in tailored voltage waveforms for capacitively coupled plasmas
- Bruneau Bastien
- Novikova T.
- Lafleur Trevor
- Booth Jean-Paul
- Johnson E.V.
Plasma Sources Science and Technology, IOP Publishing, 2015, 24 (1), pp.015021. Through the use of particle-in-cell simulations, we study the ion flux asymmetry in an argon discharge that is induced by a ?sawtooth-like? excitation voltage waveform. In a previous article we have shown that, due to their differing rising and falling slopes, these waveforms can create a plasma with a significantly higher ion flux to one electrode in a geometrically symmetric reactor. Furthermore, they have the unique property of providing a lower ion energy at the electrode with a higher ion flux. In the present work, we show that a refined waveform allows the ion flux asymmetry to be increased for a given number of harmonics by reducing the ionization rate in front of the low-flux electrode. The flux asymmetry is found to disappear at low pressure due to the increased electron energy transport, which causes a transition from sheath edge ionization to bulk ionization. Changing the fundamental frequency is shown to have two counterbalancing effects: reducing the ionization on the low ion-flux electrode and shifting the maximum ionization to the center of the discharge. Under the representative conditions that we have studied, a maximum asymmetry is found for a base frequency of 3.4 MHz. Finally, it is shown that, by adjusting the rise- to fall-time ratio of the refined waveforms, the ion-flux asymmetry can be continuously shifted from one electrode to the other. (10.1088/0963-0252/24/1/015021)
DOI : 10.1088/0963-0252/24/1/015021

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